Macquarie University
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Optical and plasmonic coupling in linear and nonlinear regimes

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posted on 2022-03-28, 21:30 authored by Vincent Ng
Surface plasmon polaritons are electromagnetic surface waves that may be excited at the interface between metallic and dielectric materials. They confine light to subwavelength dimensions, and provide large field enhancement, making them useful for creating compact devices and sensing applications. Unfortunately, surface plasmons are difficult to utilise due to their characteristically large losses. They typically have propagation lengths from microns to hundreds of microns. Surface plasmon-to-optical coupling is also challenging, due to the inherent disparity in the size and wavevector of optical and plasmonic modes. In this thesis,we take two approaches to addressing these challenges. The first approach is to explore second-order nonlinear effects. Nonlinear effects benefit from the plasmon field-enhancement, and can potentially be used to provide gain via parametric amplification. In our study, we experimentally consider the nonlinearity of gold in plasmon-to-plasmon second harmonic generation, as well as the dielectric nonlinearity in lithium niobate. In gold-coated lithium niobate crystals, we explore optical-to-plasmonic processes, using quasi-phase-matching for second harmonic generation, and birefringent phase-matching for parametric down conversion. We find that the large size disparity in optical and plasmonic modes strongly inhibits the efficiency of the nonlinear response, and diminishes the contributions made by phase-matching. We were unable to overcome the plasmonic absorption losses using second-order nonlinear effects in the nanosecond domain. In our second approach, we consider directional coupling between optical and longrange surface plasmon waveguides using numerical methods. We then consider the design of a three-waveguide device, an adiabatic passage coupler with a plasmonic intermediate waveguide. By the use of a dark state, we show that light can be transported through the plasmonic waveguide without suffering plasmonic loss. This is achieved by supressing the surface plasmon amplitude. An analogous device, a digitised adiabatic passage coupler, is characterised experimentally, verifying the tolerance to loss in that design.


Table of Contents

1. Introduction -- 2. Surface Plasmons : background and methods -- 3. Plasmonic second harmonic generation -- 4. Phase-matched plasmonic generation using dielectric nonlinearities -- 5. Photonic-plasmonic directional couplers -- 6. Plasmonic-photonic couplers based on spatial adiabatic passage -- 7. Conclusion and future work -- Appendices -- References.


Thesis by publication. Bibliography: pages 145-161

Awarding Institution

Macquarie University

Degree Type

Thesis PhD


PhD, Macquarie University, Faculty of Science and Engineering, Department of Physics and Astronomy

Department, Centre or School

Department of Physics and Astronomy

Year of Award


Principal Supervisor

Judith M. Daes

Additional Supervisor 1

D. W. (David William) Coutts


Copyright Vincent Ng 2018. Copyright disclaimer:






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